@article{8bdc34fe43b34daf95c1cd6bacd0a1e2,
title = "2D Undulated Metal Hydrogen-Bonded Organic Frameworks with Self-Adaption Interlayered Sites for Highly Efficient C–C Coupling in the Electrocatalytic CO2 Reduction",
abstract = "Highly crystalline 2D metal hydrogen-bonded organic frameworks (2D-M-HOFs) including 2D-Cu-HOF and 2D-Ni-HOF were designed and synthesized. The 2D-M-HOF with flexible ligands leads to the formation of the self-adaption interlayered sites, which facilitate the C–C couple and overcome the limitations of the coadsorption of multiple intermediates in the electrocatalytic CO2 reduction reaction. The undulated 2D-Cu-HOF exhibits outstanding activity and selectivity for electrocatalytic reduction of CO2 to C2 products with a total Faradaic efficiency of 82.1\% (48.2\% for C2H5OH and 33.9\% for C2H4) at −1.2 V vs. RHE.",
keywords = "Electrocatalytic CO reduction, Flexible structure, Hydrogen-bonded organic frameworks, Self-adaption interlayered sites",
author = "Jianning Lv and Wenrui Li and Shuai Li and Shuo Xu and Zunhang Lv and Zhejiaji Zhu and Lu Dai and Bo Wang and Pengfei Li",
note = "Publisher Copyright: {\textcopyright} The Author(s) 2025.",
year = "2025",
month = dec,
doi = "10.1007/s40820-025-01679-3",
language = "English",
volume = "17",
journal = "Nano-Micro Letters",
issn = "2311-6706",
publisher = "Open Access Science Online",
number = "1",
}